Just a quick sanity check here:
I'm preparing a tutorial for a class on classical electrodynamics and I wanted to show an example of a gauge condition which leads to a contradiction, so I simply thought of $$(A^\mu)' = A^\mu - \partial^\mu \chi \stackrel{!}{=} 0\quad \forall \mu \in \{0,1,2,3\}\qquad (1)$$ For the 0th component this gives me the Weyl gauge ($\phi = 0$), which is allowed since I will always find a $\chi$ satisfying $$\phi = \frac1c \partial_t\chi.$$ I do, however, have a contradiction in the spatial components, since $$\vec{A} = \vec{\nabla}\chi$$ is only true for $\vec{A}$ with $\vec{\nabla}\times\vec{A}=0$ (on a simply-connected region), so if a given vector potential has non-vanishing rotation, I won't be able to find a $\chi$ so that the transformed field vanishes in all components.
Does anyone have some other examples?
(1) - As mentioned by QMechanic: Here are actually four gauge-fixing conditions disguised as one; this is unusual since common gauges (e.g. $\vec{\nabla}\cdot\vec{A}=0$) generally eliminate only one degree of freedom.