The definition of angle of declination is the angle between the geometric meridian and the magnetic meridian. You can look up the exact definition in words on wikipedia, but there is a easier way to visualise it. Firstly, we should know that the magnetic poles are a bit tilted to the actual geometric north and south poles.
Imagine you are a sailor. You are in the nothern hemisphere and want to go to the geometric North pole. If you use a compass, it will take you to the magnetic North pole instead of the geometric pole. The angle of declination is nothing but the angle between these two paths.
Image for reference:
These paths are curved due to the Earth's curvature. Therefore, these paths will not be 1 dimensional, but 2-dimensional. There are two points on the earth, A and B which are your positions(as a sailor). Here's the fun part: $\alpha$ and $\beta$ are angle of declinations! Why? Because if you are are position A, then the 2-D paths show us the planes. Path A to Geometric North is geometric meridian, while Path A to Magnetic North is magnetic meridian.
Now, it is easier to say that as you move away from the poles, the angle of declination decreases, because angle subtended by two far away points is less than two closer points. Therefore $\beta$ is less than $\alpha$.
Hence, then declination angle increases as we move closer to the poles.
IMPORTANT: However, this was a general case explanation. The angle of declination not only depends on the lattitude, but also the longitude. If the paths to geometric north and magnetic north coincide, then the angle of declination will be 0 irrespective of the lattitude.
It is just generally said that at higher lattitude, the angle of declination is higher, but obviously, yes it will depend on the longitude as well.
Conclusion: You cannot be sure whether the angle of declination will increase or decrease just by knowing the lattitudes. You should also have some information about the longitudees too, to know for sure