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I was wondering whether dual large angle scattering and multiple small angle scattering is of great significance in proton colision with light nuclei in comparison to heavy nuclei.

For instance given the elastic scattering of protons from Boron $^{nat}B(p,p)^{nat}B$ and the elastic scattering of protons from a heavier nuclei(i.e. Phosphorus) which reaction has larger significance in multiple and dual scattering?

I was thinking that when protons colliding with a lighter nuclei, they will lose their energy in fewer collision steps in comparison with a heavier nuclei scattering, but I can't think of how this will affect the energy straggling.

Any idea or reference to that?

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  • $\begingroup$ I'm a little unclear on what you are asking. Assuming generally Rutherford cross sections, it is a tradeoff between greater energy transfer to a light nucleus (goes as $4m_{1}m_{2}/(m_{1}+m_{2})^2$) vs the increase in cross section for heavier nuclei that goes as $Z^2$. I'm assuming energetic protons into a solid material? Ignoring channeling issues as well. Is that generally what you want? $\endgroup$
    – Jon Custer
    Commented Sep 17, 2014 at 14:04
  • $\begingroup$ @JonCuster : Thank's for your comment! Ignoring channeling effects for sure. Protons of energy in the range 2-3 MeV. $\endgroup$
    – Thanos
    Commented Sep 17, 2014 at 14:58

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I think I've get a better idea of what you are looking for now, thanks.

As background for others in the future: classic ion-solid interaction theory dates back to the 1960s and is commonly called LSS theory after Linhard, Scharff, and Schiott who first formulated the concepts. It splits the energy loss mechanisms of the ion into two components, electronic stopping (ion-electron interactions), and nuclear stopping (ion-nuclei interactions). There are many ion-electron interactions, and the maximum energy transferred by any one of them is small, so this acts generally as a viscous drag force on the ion, giving an increasing angular spread to the beam as it travels through the solid. The ion-nuclei interactions are what Geiger and Marsden saw: Rutherford scattering. The larger the scattering angle, the greater the energy transferred to the nucleus from the incident ion (simple kinematics).

LSS theory allows one to calculate the range and distributions for ions implanted into solids. Many folks use SRIM from John Ziegler (srim.org) to get range, stopping, and perform simulations of ion implants. Note one should take the absolute numbers from SRIM with at least a grain of salt, since it doesn't handle channeling effects.

For MeV H into almost any material, the overwhelming energy loss mechanism, on average, is electronic stopping. From SRIM one can get that 99+% of the energy loss of 2MeV hydrogen into B, P, or Au is ionization (electronic stopping) as averaged over many incident ions. Those nuclei are small! Nuclear cross sections are measured in barns, or $10^{-24} cm^2$.

As an example: MeV H or He is regularly used in Rutherford Backscattering Spectrometry (RBS) for materials composition analysis of thin films. Often one uses about 20nC of ions, which is about 125,000,000 ions hitting the film. Not that many bounce back. A (simplified) equation for the differential Rutherford cross section comes from Chu, Mayer, and Nicolet, 'Backscattering Spectrometry' (1979). It is:

$\sigma(\theta) = ({{Z_{1}Z_{2}e^{2}} \over {2E_{0}}})^{2} {{(cos(\theta) + \sqrt{1-x^{2} sin^{2}(\theta)}})^{2} \over sin^{4}(\theta)\sqrt{1-x^{2} sin^{2}(\theta)}}$

where $x = m_{1}/m_{2}$ and $E_0$ is the incident energy. This is in units of barns/steradian (cross section to be deflected into solid angle at $\theta$, in lab coordinates).

How big are these numbers? Well, for 1MeV H on B, $\sigma(175^{\circ}) = 0.0319$ barns. For fun I'll plot the Rutherford cross sections for 2MeV H onto B, P, and Au: Rutherford Cross Sections for 2MeV H

Large recoil angles are large energy transfers to the target nucleus. As you can see, such large transfers are much much much less likely than small energy transfers at these energies. Now, as the incident ion loses energy (through electronic or nuclear stopping), you can see from the formula that the cross sections go up. Near the end of range, multiple nuclear collisions become fairly normal, but the total energy transferred is pretty low (remember, 99+% of the incident H energy is going into electronic stopping).

So, multiple high-energy-transfer collisions are only likely at low ion energy, i.e. already near their end of travel - such multiple scatterings should not dramatically affect the straggle. This is caused much more by spreading from electronics stopping, a few low angle collisions, and a very few high angle collisions. (Now, lower energy heavy ions, such as 100keV Au->Au will show multiple large-angle collisions since the cross sections are much bigger).

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  • $\begingroup$ Thank you very much for your answer! To sum up, you wouldn't consider dual and multiple scattering important, thus you wouldn't include it in a simulation? $\endgroup$
    – Thanos
    Commented Sep 18, 2014 at 6:19
  • $\begingroup$ For MeV light ions (H, He), I would not worry about multiple scattering - that is correct. $\endgroup$
    – Jon Custer
    Commented Sep 18, 2014 at 12:58

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