Define $$n_r~:=~n-\ell-1~\geq 0,$$ where $n$ and $\ell$ is the principalprincipal and azimuthalazimuthal quantum number, respectively. Bohr's modelBohr's model works best in the limit
$$ \ell \gg 1 $$
(to get to the semiclassical limitsemiclassical limit & the correspondence principlecorrespondence principle), and
$$ n_r \text{ small} $$
(to ensure that the orbital has a well-defined radius).