Compact group $SU(2)$ really has only finite-dimensional unitary irreducible representations, but
formally it is not enough to close the question, because there are unitary irreducible infinite-dimensional representations of spin group $SL(2,C)$ of four-dimensional relativistic Lorentz group and they were used in some models, below is a cite from: N.N. Bogolubov, A. A. Logunov, A.I. Oksak, I. Todorov, General principles of quantum field theory, Springer, 1989. Appendix I for chapter 9
The concept of an infinite-component
field (ICF for short) is the result of
abandoning the "technical" requirement
that the representations of the
Lorentz group according to which the
fields transform (say, in the Wightman
formalism) be finite-dimensional. This
idea turned up at the earliest stages
of quantum field theory: in 1932,
Majorana gave an example of an
infinite-dimensional wave equation
$(i \Gamma^\mu \partial_\mu – M) \psi(x) = 0$
without negative-energy solutions
of non-negative square mass, that is,
without "antiparticles".
…
Running ahead (see
§1.3), it should be noted, however,
that the description of composite
systems by means of ICF's has met with
difficulties which, it would seem,
require a weakening of the postulate
of (strict) locality.